A long excitation coil piercing a superconducting ring is used to generate an ever increasing persistent current in the ring, until the current destroys the order parameter. Given that the penetration depth $\lambda$ is known, this experiment measures, hypothetically, the coherence length $\xi$. We examine various aspects of this theoretically driven hypothesis by testing niobium rings with different dimensions, and by comparing the results to the known values of $\xi$. We then apply the method to two ${\mathrm{La}}_{1.875}{\mathrm{Sr}}_{0.125}{\mathrm{CuO}}_4$ rings at $T\to 0$. In one, the current flows in the ${\mathrm{CuO}}_2$ planes, hence it is set by ${\xi }_{ab}$. In the other, the current must cross planes and is determined by ${\xi }_c$. We find that ${\xi }_c=1.3\pm 0.1$ nm, and ${\xi }_{ab}<2.3\mathrm{nm}$, indicating that at low temperatures the Cooper pairs are three dimensional.

Heterostructures in nanoparticles challenge our common understanding of interfaces due to quantum confinement and size effects, giving rise to synergistic properties. An alternating heterostructure in which multiple and reoccurring interfaces appear in a single nanocrystal is hypothesized to accentuate such properties. We present a colloidal synthesis for perovskite layered heterostructure nanoparticles with a (PbBr₂)₂(AMTP)₂PbBr₄ composition. By varying the synthetic parameters, such as synthesis temperature, solvent, and selection of precursors, we control particle size, shape, and product priority. The structures are validated by X-ray and electron diffraction techniques. The heterostructure nanoparticles’ main optical feature is a broad emission peak, showing the same range of wavelengths compared to the bulk sample.

Bosonic encoding is an approach for quantum information processing, promising lower hardware overhead by encoding in the many levels of a harmonic-oscillator mode. Scaling to multiple modes requires weak interaction for independent control, yet strong interaction for fast control. Applying fast and efficient universal control on multiple modes remains an open problem. Surprisingly, we find that displacements conditioned on the state of a single-qubit ancilla coupled to multiple harmonic oscillators are sufficient for universal control. We present the conditional-no operation concept, which can be used to reduce the duration of entangling gates. Within this guiding concept, we develop the conditional-not displacement control method which enables fast generation and control of bosonic states in multimode systems weakly coupled to a single-ancilla qubit. Our method is fast despite the weak ancilla coupling. The weak coupling in turn allows for excellent separability and thus independent control. We demonstrate our control on a superconducting transmon qubit weakly coupled to a multimode superconducting cavity. We create both entangled and separable cat states in different modes of the multimode cavity, showing entangling operations at low crosstalk while maintaining independent control of the different modes. We show that the operation time is not limited by the inverse of the coupling rate, which is the typical timescale, and we exceed it by almost 2 orders of magnitude. We verify our results with an efficient method for measurement of the multimode characteristic function which employs our conditional-not displacement. Our results inspire a new approach toward general entangling operations and allow for fast and efficient multimode bosonic encoding and measurement.

The problem of quantum measurement can be partially resolved by incorporating a process of spontaneous disentanglement into quantum dynamics. A modified master equation is proposed, which contains a nonlinear term giving rise to both spontaneous disentanglement and thermalization. It is found that the added nonlinear term enables limit cycle steady states, which are prohibited in standard quantum mechanics. This finding suggests that an experimental observation of such a limit cycle steady state can provide an important evidence supporting the spontaneous disentanglement hypothesis.

We observe non-perturbative high harmonic generation in solids pumped by a macroscopic quantum state of light, bright squeezed vacuum (BSV), which we generate in a single spatiotemporal mode. Due to its broad photon-number distribution, covering states from $0$ to $2 \times 10^{13}$ photons per pulse, and sub-cycle electric field fluctuations over $\pm1\hbox{V}/\hbox{\r{A}}$, BSV provides access to free carrier dynamics within a much broader range of peak intensities than accessible with coherent light. It is also considerably more efficient in the generation of high harmonics than coherent light of the same mean intensity.

Integrating light emitters based on III-V materials with silicon-based electronics is crucial for further increase in data transfer rates in communication systems since the indirect bandgap of silicon prevents its direct use as a light source. We investigate here InAs/InGaAlAs quantum dot (QD) structures grown directly on 5{\deg} off-cut Si substrate and emitting light at 1.5 micrometers, compatible with established telecom platform. Using different dislocation defects filtering layers, exploiting strained superlattices and supplementary QD layers, we mitigate the effects of lattice constant and thermal expansion mismatches between III-V materials and Si during growth. Complementary optical spectroscopy techniques, i.e. photoreflectance and temperature-, time- and polarization- resolved photoluminescence, allow us to determine the optical quality and application potential of the obtained structures by comparing them to a reference sample -- state-of-the-art QDs grown on InP. Experimental findings are supported by calculations of excitonic states and optical transitions by combining multiband k.p and configuration-interaction methods. We show that our design of structures prevents the generation of a considerable density of defects, as intended. The emission of Si-based structures appears to be much broader than for the reference dots, due to the creation of different QD populations which might be a disadvantage in particular laser applications, however, could be favourable for others, e.g. in broadly tunable devices, sensors, or optical amplifiers. Eventually, we identify the overall most promising combination of defect filtering layers, discuss its advantages and limitations, and prospects for further improvements.

Electrical doping of semiconductors is a revolutionary development that enabled many electronic and optoelectronic technologies. While doping of many inorganic and organic semiconductors has been well-established, controlled electrical doping of metal halide perovskites is yet to be demonstrated. In this work, we achieve efficient n- and p-type electrical doping of metal halide perovskites by co-evaporating the perovskite precursors alongside organic dopant molecules. We demonstrate that the Fermi level can be shifted by up to 500 meV towards the conduction band and by up to 400 meV towards the valence band by n- and p-doping, respectively, which increases the conductivity of the films. The doped layers were employed in PN and NP diodes, showing opposing trends in rectification. Demonstrating controlled electrical doping by a scalable, industrially relevant deposition method opens the route to developing perovskite devices beyond solar cells, such as thermoelectrics or complementary logic.

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We have successfully demonstrated the first CMOS-compatible monolithic epitaxial integration of GaN-based infrared (IR) detectors on Si. The device is a GaN/AlGaN quantum cascade detector (QCD) grown selectively in windows on a 4-in Si (111) substrate using plasma-assisted molecular beam epitaxy. The CMOS compatibility of the QCD growth method was verified by applying it to Si circuitry fabricated on (100) surface of a double hetero-oriented silicon on insulator (SOI) substrate. The photo signal, centered at a wavelength of 4.6 $\mu$ m, was measured at 110 K. The zero-bias responsivity of 81 $\mu$ A/W at 18 K and detectivity of 1.2 $\times$ 10 $^{\text{7}}$ Jones were recorded.

Cluster states are key resources for measurement-based quantum information processing. Photonic cluster and graph states, in particular, play indispensable roles in quantum network and quantum metrology. We demonstrate a semiconductor quantum dot based device in which the confined hole spin acts as a needle in a quantum knitting machine producing continuously and deterministically at sub-Gigahertz repetition rate single indistinguishable photons which are all polarization entangled to each other and to the spin in a one dimensional cluster state. By projecting two nonadjacent photons onto circular polarization bases we disentangle the spin from the photons emitted in between, thus continuously and deterministically preparing all-photonic cluster states for the first time. We use polarization tomography on four sequentially detected photons to demonstrate and to directly quantify the robustness of the cluster's entanglement and the determinism in its photon generation.

Cavity QED, wherein a quantum emitter is coupled to electromagnetic cavity modes, is a powerful platform for implementing quantum sensors, memories, and networks. However, due to the fundamental trade-off between gate fidelity and execution time, as well as limited scalability, the use of cavity QED for quantum computation was overtaken by other architectures. Here, we introduce a new element into cavity QED—a free charged particle, acting as a flying qubit. Using free electrons as a specific example, we demonstrate that our approach enables ultrafast, deterministic, and universal discrete-variable quantum computation in a cavity-QED-based architecture, with potentially improved scalability. Our proposal hinges on a novel excitation blockade mechanism in a resonant interaction between a free-electron and a cavity polariton. This nonlinear interaction is faster by several orders of magnitude with respect to current photon-based cavity-QED gates, enjoys wide tunability and can demonstrate fidelities close to unity. Furthermore, our scheme is ubiquitous to any cavity nonlinearity, either due to light-matter coupling as in the Jaynes-Cummings model or due to photon-photon interactions as in a Kerr-type many-body system. In addition to promising advancements in cavity-QED quantum computation, our approach paves the way towards ultrafast and deterministic generation of highly entangled photonic graph states and is applicable to other quantum technologies involving cavity QED.