Quantum tunnelling of electrons can be confined to the sub-cycle time scale of strong light fields, contributing decisively to the extreme time resolution of attosecond science. Because tunnelling also enables atomic-scale spatial resolution in scanning tunnelling microscopy (STM), integrating STM with light pulses has long been a key objective in ultrafast microscopy, spanning the picosecond and femtosecond domains, with first signatures of attosecond dynamics. However, while sub-cycle dynamics on the attosecond time scale are routinely controlled and determined with high precision, controlling the direction of attosecond currents and determining their duration have remained elusive in STM. Here, we induce STM tunnelling currents using two-colour laser pulses and dynamically control their direction, relying solely on the sub-cycle waveform of the pulses. Projecting our measurement data onto numerical and analytical solutions of the time-dependent Schr\"odinger equation reveals non-adiabatic tunnelling as the underlying physical mechanism, yielding a current burst duration of 860 as. Despite working under ambient conditions but free of thermal artifacts, we achieve sub-angstr\"om topographic sensitivity and a lateral spatial resolution of 2 nm. This unprecedented capability to directionally control attosecond bursts will enable triggering and imaging ultrafast charge dynamics in atomic, molecular and condensed systems at the spatio-temporal microscopy frontier of lightwave electronics.

Beam dump experiments represent an effective way to probe new physics in a parameter space, where new particles have feeble couplings to the Standard Model sector and masses below the GeV scale. The LUXE experiment, designed primarily to study strong-field quantum electrodynamics, can be used also as a photon beam dump experiment with a unique reach for new spin-0 particles in the $10-350~\mathrm{MeV}$ mass and $10^{-6}-10^{-3}~\mathrm{GeV}^{-1}$ couplings to photons ranges. This is achieved via the ``New Physics search with Optical Dump'' (NPOD) concept. While prior estimations were obtained with a simplified model of the experimental setup, in this work we present a systematic study of the new physics reach in the full, realistic experimental apparatus, including an existing detector to be used in the LUXE NPOD context. We furthermore investigate updated scenarios of LUXE's experimental plan and confirm that our results are in agreement with the original estimations of a background-free operation.

The Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) theory successfully explains the melting mechanism of two-dimensional isotropic lattices as a two-step process driven by the unbinding of topological defects. By considering the elastic theory of the square lattice, we extend the KTHNY theory to melting of square lattice solids. In addition to the familiar elastic constants that govern the theory -- the Young's modulus and the Poisson ratio -- a third constant controlling the anisotropy of the medium emerges. This modifies both the logarithmic and angular interactions between the topological defects. Despite this modification, the extended theory retains the qualitative features of the isotropic case, predicting a two-step melting with an intermediate tetratic phase. However, some subtle differences arise, including a modified bound on the translational correlation exponent and the absence of universal values for the Young's modulus at the solid-to-tetratic phase transition.

Material research is a key frontier in advancing superconducting qubit and circuit performance. In this work, we develop a simple and broadly applicable framework for accurately characterizing two-level system (TLS) loss using internal quality factor measurements of superconducting transmission line resonators over a range of temperatures and readout powers. We applied this method to a series of $\alpha$-Ta resonators that span a wide frequency range, thus providing a methodology for probing the loss mechanisms in the fabrication process of this emerging material for superconducting quantum circuits. We introduce an analytical model that captures the loss behavior without relying on numerical simulations, enabling straightforward interpretation and calibration. Additionally, our measurements reveal empirical frequency-dependent trends in key parameters of the model, suggesting contributions from mechanisms beyond the standard tunneling model of TLSs.

Over the past century, continuous advancements in electron microscopy have enabled the synthesis, control, and characterization of high-quality free-electron beams. These probes carry an evanescent electromagnetic field that can drive localized excitations and provide high-resolution information on material structures and their optical responses, currently reaching the sub-Å and few-meV regime. Moreover, combining free electrons with pulsed light sources in ultrafast electron microscopy adds temporal resolution in the subfemtosecond range while offering enhanced control of the electron wave function. Beyond their exceptional capabilities for time-resolved spectromicroscopy, free electrons are emerging as powerful tools in quantum nanophotonics, on par with photons in their ability to carry and transfer quantum information, create entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena. This Roadmap outlines the current state of this rapidly evolving field, highlights key challenges and opportunities, and discusses future directions through a collection of topical sections prepared by leading experts.

The gas-phase hydrogen exchange reaction (HER) is the most fundamental chemical process for benchmarking quantum reaction dynamics. In this Letter, we focus on controlling HER by means of strong light-matter coupling inside a resonant cavity, an approach often called polariton chemistry. In particular, we focus on the isotopic variation of HER involving collisions between molecular hydrogen H$_2$ and deuterium atom D, i.e., H$_2$+D$\to$HD+H. We find that the asymmetry introduced by the different isotopes, despite being small, enables strong cavity-induced modifications of reaction rates. Outside of the cavity the reaction is as usual D+H${_2}$$\to$DH+H. However, inside the cavity another type of reactions take place where D+H$_2$$\to$DH+H+E$_{photon}$, where E$_{photon}$=$\hbar\omega_{cav}$. Our results show that HER is an ideal platform to make a significant step toward closing the gap between theory and experiment in polariton chemistry.

Quantum metrology experiments in atomic physics and quantum optics have demonstrated measurement accuracy beyond the shot-noise limit via multi-particle entanglement. At the same time, electron microscopy, an essential tool for high-resolution imaging of biological systems, is severely constrained in its signal-to-noise ratio (SNR) by shot noise, due to the dose limit imposed by electron beam-induced damage. Here, we show theoretically that spin squeezing, a form of quantum metrology based on entanglement, is a natural fit for improving the SNR in electron microscopy. We investigate the generation of the necessary entangled states through electron-electron Coulomb interactions and quantum non-demolition measurements. Our results connect the fields of quantum metrology and electron interferometry, paving the way toward electron microscopy with SNR beyond the shot-noise limit.

Correlated topological materials often maintain a delicate balance among physical symmetries. Many topological orders are symmetry protected, whereas most correlated phenomena arise from spontaneous symmetry breaking. Cases where symmetry breaking induces a non-trivial topological phase are rare. Here we demonstrate the presence of two such phases in Ta₂Pd₃Te₅, where Coulomb interactions form excitons that condense below 100 K, one with zero and the other with finite momentum. We observed a full spectral bulk gap, which stems from exciton condensation. This topological excitonic insulator state spontaneously breaks mirror symmetries but involves a weak structural coupling. Scanning tunnelling microscopy shows gapless boundary modes in the bulk insulating phase. Their magnetic field response, together with theoretical modelling, indicates a topological origin. These observations establish Ta₂Pd₃Te₅ as a topological excitonic insulator in a three-dimensional crystal. Thus, our results manifest a unique sequence of topological exciton condensations in a bulk crystal, offering exciting opportunities to study critical behaviour and excitations.

We show how amplitude modulated, coherent high-frequency drives can be used to access otherwise difficult to reach collective resonances and off-resonantly induce parametric instabilities. In particular, we demonstrate that difficult to access antiferromagnetic resonances in the THz range can be parametrically excited with signals at optical frequencies via a mechanism that we call Modulated Floquet Parametric Driving (MFPD). We study spin pumping and the formation of entangled, two-mode squeezed magnon pairs in anisotropic antiferromagnets under MFPD. Furthermore, we show that MFPD induces transitions to symmetry breaking steady-states in which dynamical spin patterns are formed by resonant magnon pairs.

This paper presents a novel continuous-flow electron spin resonance (ESR) microfluidic device designed for both continuous-wave (CW) and pulsed ESR measurements on sub-nanoliter liquid samples. The system integrates a planar surface microresonator (ParPar type) operating at ∼9.4 GHz with a precision-fabricated quartz microfluidic chip, enabling spatial confinement of the sample within the resonator’s microwave magnetic field hotspot while minimizing dielectric losses. The effective sample volume is ∼0.06 nL, and the device supports standard microfluidic connectors, facilitating both continuous and stopped-flow experiments. Using a 1 mM aqueous solution of deuterated Finland trityl (dFT) radical, CW ESR measurements yielded a peak signal-to-noise ratio (SNR) of ∼83 for a 100-point spectrum acquired over 80 s, with a resonator quality factor of Q ∼15–20. This corresponds to a spin sensitivity of ∼1.04 × 10⁹ spins/√Hz/G. Pulsed ESR measurements, performed with 0.1 W microwave power and 10 ns π pulses, achieved an SNR of ∼47 with 1 s of averaging, corresponding to a spin sensitivity of ∼7.8 × 10⁸ spins/√Hz. A Rabi frequency of ∼50 MHz was measured, indicating a microwave conversion efficiency of ∼56 G/√W. Both the pulsed spin sensitivity and Rabi frequency are consistent with simulated values. This device represents a significant step toward ESR-based detection of individual, slowly flowing cells—analogous to flow cytometry but with magnetic resonance contrast. With future enhancements such as higher operating frequencies, cryogenic integration, or optimized resonator geometries, the system is expected to enable practical ESR measurements at the single-cell level.